分类： 核科学技术 >> 核材料与工艺技术 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
LAN Tu
DING Cong-Cong
LIAO Jia-Li
LI Xiao-Long
LI Xing-Liang
ZHANG Jie
ZHANG Dong
YANG Ji-Jun
LUO Shun-Zhong
AN Zhu
WU Qi-Qi
YANG Yuan-You
FENG Su
TANG Jun
LIU Ning
摘要： To develop a microbe-based bioremediation strategy for cleaning up thorium-contaminated sites, we have investigated the biosorption behavior and mechanism of thorium on Bacillus sp. dwc-2, one of the dominant species of bacterial groups isolated from soils in Southwest China. Thorium biosorption depended on the pH of environment, and its rapid biosorption reached a maximum of up to 10.75 mg Th per gram of the bacteria (wet wt.) at pH 3.0. The biosorption agreed bettter with Langmuir isotherm model than Freundlich model, indicating that thorium biosorption was a monolayer adsorption. The thermodynamic parameters, negative change in Gibbs free energy and positive value in enthalpy and entropy, suggested that the biosorption was spontaneous, more favorable at higher temperature and endothermic process with an increase of entropy. Scanning electron microscopy (SEM) indicated that thorium initially binded with the cell surface, while transmission electron microscopy (TEM) revealed that Th deposited in the cytoplasm and served as cores for growth of element precipitation (e.g., phosphate minerals) or by self-precipitation of hydroxides, which is probably controlled by ion-exchange, as evidenced by particle induced X-ray emission (PIXE) and enhanced proton backscattering spectrometry (EPBS). Fourier Transform Infrared (FTIR) further indicated that thorium biosorption involved carboxyl and phosphate groups and protein in complexation or electrostatic interaction. Overall results indicated that a combined electrostatic interaction-complexation-ion exchange mechanism could be involved in thorium biosorption by Bacillus sp. dwc-2.
分类： 核科学技术 >> 核探测技术与核电子学 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： In this paper, we present a novel method for digital nuclear signal processing based on image processing and recognition, which can improve signal-to-noise ratio of digital nuclear signal effectively without changing the signal shape. The digital nuclear signal with a time-amplitude series is converted into a grayscale image with adjustable pixel size. Template of the converted image is extracted by means of modern image processing methods, such as spatial digital low-pass filtering, image binary and the skeleton extracting of images. The needed parameters are extracted from the template image. The method of template extracting presented in this paper can be used flexibly to extract template of nuclear signals, whether the whole or even part of that, and got multi templates corresponding to the whole or partial characters of the signals. The results of image processing, along with -ray energy spectrum of 241Am acquired by this method, show that the new method provides a way to develop future digital nuclear instruments of high efficiency and flexibility, high density and multi parameters.
分类： 核科学技术 >> 核探测技术与核电子学 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： A principle and method of constructing the digital acquisition system is presented in this work, which is convenient for the study on the theories and algorithms of digital nuclear signal processing. The hardware system of the digital acquisition system consists of front-end controller, waveform digitizer and PC workstation, on which the software system has been developed based on Visual C++ under Windows environment. The alterable-frequency sampling (AFS) algorithm and the alterable-frequency trapezoidal filter (AFTF) algorithm have also been studied in the real-time environment, along with a digital nuclear spectrum acquisition system being set up based on the new algorithms and the -ray spectra of 241Am being shown. A useful experimental platform could be provided by this work for the successive work such as the development of global digitized nuclear measurement system and the study of digital nuclear signal processing.
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